George William Spencer Lyttelton was born in Westminster, London on 12 June 1847, the fourth son of George Lyttelton, 4th Baron Lyttelton and his first wife Mary Glynne. Having studied at Eton College, he attended Trinity College, Cambridge, from which he graduated with a Bachelor of Arts in 1869 and received his Master of Arts in 1874. He played a number of cricket matches for Eton during his time at the school, including the annual fixture against Harrow in each of 1863, 1864 and 1865. In his first of these contests, he claimed four wickets in Harrow's only batting innings of a drawn match, and he scored a half-century in the second, but could not prevent Eton losing by an innings that year. In both of these contests, he played alongside his older brother Neville. In his final year at Eton, he was the captain of the cricket team. In the match against Harrow that year, in which Lyttelton claimed three wickets, his side once again lost by an innings. He made his first-class debut during his first year at Cambridge; appearing against the Marylebone Cricket Club in May 1866. He claimed a wicket in each innings, and scored 23 runs in his only appearance at the crease. Facing Cambridgeshire later that month, he took seven wickets in the first innings, conceding 33 runs; the best bowling figures of his career. He collected three further wickets in the second innings to complete the only ten wicket haul of his career. He received his blue that year by appearing in the match against Oxford. He made scores of one and three with the bat, and took three tail-end wickets in a match which Cambridge lost by 12 runs. Despite his bowling achievements in 1866, in which he claimed 16 wickets for Cambridge at an average of 14.75, he was used as wicket-keeper for his first appearance in the subsequent year, taking five stumpings against the MCC. In the next match, against Southgate, he narrowly missed out on a century, having scored 99 runs in the first innings, but achieved the landmark score in the following game, against Cambridgeshire. Batting at number four, he scored 114 runs, almost half of his team's total for the first innings. The university won by eight wickets. The score remained the best of his career, resulting in both his highest total batting, and his best bowling figures, being against the same side: Cambridgeshire. He represented his university against Oxford for the second and final time in 1867, and though he claimed just one wicket and made scores of 17 and 20 not out, he was praised for his sensible batting in the second innings which helped his team win the match by five wickets. In 1868, Lyttelton played five matches for Cambridge, but did not feature in the contest with Oxford. His batting average dropped significantly from the previous year's 37.88 to 13.57, and over half of his wickets for the season came in a match against Southgate. In that match he took five wickets for 17 runs in the second innings, the second five-wicket haul of his career. After leaving university, Lyttelton only played two further first-class matches, appearing for the amateur side "Gentlemen of England" against a university on each occasion. Along with the majority of his family, he appeared a number of times for the "Gentlemen of Worcestershire", a fore-runner to Worcestershire County Cricket Club, for whom he made his debut in a match against the "Gentlemen of Warwickshire" shortly before entering Cambridge. Playing for the county in 1866, Lyttelton and his brother Charles took nine of Shropshire's first innings wickets, the other being a run out. In 1878, six years after his final first-class appearance, he scored 127 runs against the Free Foresters, his highest recorded batting total for the county. E.F. Benson described him as "grim and blunt and bearded and rich: he lived alone in a house in Hill Street into which no friend had ever penetrated. He was a bachelor, he sang in the Bach choir, and on being asked if had ever in his life kissed a woman he replied: "Once. On the brow."