The formation of Land and Liberty, in Saint Petersburg in 1876, was preceded by the analysis of the "call to the people" campaign of 1873-1875. As a result, the members of Land and Liberty defined the basics of the political platform, which would be called narodnicheskaya. They admitted a possibility of a special, non-capitalist way of development of Russia with peasantry as its basis. The members of Land and Liberty considered necessary to adapt the purposes and slogans of the movement to independent revolutionary aspirations that had already existed among the peasants, as they believed. These requirements, generalized in the slogan "Land and Liberty!", were designed to allow for the transition of all the lands "into the hands of the rural working ", even distribution of the land, "full communal self-management" and division of the Russian empire into parts "in accordance with the desires of the locals". Land and Liberty stood for the creation of permanent "revolutionary settlements" in the countryside for the purpose of preparing a people’s revolution. The members of Land and Liberty saw peasantry as the principal revolutionary force, as opposed to the working class, which would have to play a part of the "second fiddle". Proceeding from the inevitability of a "forced coup d'état", the revolutionaries considered agitation and organization of revolts, demonstrations and strikes to be very important. Land and Liberty represented a "rebellious" current of the revolutionary movement of the 1870s. Vladimir Lenin said that Land and Liberty’s merit was its desire to "...attract all of the discontent and direct the organization towards decisive struggle against autocracy". Discipline, mutual comradely control, centralism and conspiracy became this organization’s principles.
The revolutionaries chose to "settle" in the provinces of Saratov, Nizhny Novgorod, Samara, Astrakhan, Tambov, Pskov, Voronezh, the Donregion and others. They also attempted to spread their revolutionary activities in the Northern Caucasus and the Urals. Land and Liberty organized clandestine publishing and distribution of the revolutionary literature, conducted propaganda among workers and took part in several strikes in Petersburg in 1878-1879. It also influenced the development of the student movement by organizing or supporting demonstrations in Petersburg and other cities, including the so-called Kazan demonstration of 1876, where they would openly admit the organization’s existence for the first time. The Program of Land and Liberty also envisioned a course of actions, aimed at "disorganization of the state", in its members opinion. In particular, it allowed for physical elimination of "the most harmful or prominent members of the government". The most famous terrorist act of Land and Liberty was the assassination of the Chief of the Gendarmes Nikolai Mezentsov in 1878. However, Land and Liberty didn’t yet consider terror a means of political struggle against the existing regime, perceiving it as revolutionary self-defense and their revenge towards the government. Land and Liberty’s disappointment with the revolutionary activity in the countryside, intensification of the governmental repressions and political discontent during the Russo-Turkish War, 1877-78 and ripening of the revolutionary situation favored the conception and development of the new sentiments in the organization itself. By spring of 1879, the faction of political terrorists was formed in Land and Liberty Disagreements between the supporters of the former strategy of inciting the countryside called derevenschiki, or "villagers" and defenders of transition towards political struggle by means of systematic terrorist methods called politicians led to the convocation of the Voronezh Congress of Land and Liberty in June 1879, where the two rival groups would reach a short-term compromise. In August 1879, however, Land and Liberty broke up in two independent organizations: Narodnaya Volya and Chernyi Peredel.
